Characterization of size resolved atmospheric particles in the vicinity of iron and steelmaking industries in China

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Abstract

(Graphical abstract)

China currently faces environmental challenges of lower air quality, partly as a result of industrial activities. The aim of this study was to investigate the role of iron and steelmaking facilities to regional air quality in four selected industry dominated urban centres in China. Nine different particle size ranges present in atmospheric particles collected from four sites in Kunming (KM), Wuhan (WH), Nanjing (NJ) and Ningbo (NB) were analysed and compared with particles collected at one background site at the Ningbo Nottingham University (UN) with very little industrial influence in China. Similar mass concentration levels of particulate matter PM2.1 and PM1.1 were found at the three sites near older iron and steelmaking plants (KM, WH and NJ). Significantly lower levels of PM2.1 and PM1.1 were collected at the fourth site (NB), which is near to a modern and coastal iron and steelmaking plant. The particles collected had the highest mass concentration in the aerodynamic diameter range of 3.3–9.0 μm for all sites, except for the background site (UN). Scanning electron microscopy equipped with energy-dispersive X-ray spectroscopy, and inductively coupled plasma were used to determine the surface morphology and particle chemistry. Al, Ca, Fe, K, Mg, Na and Zn were found as the most abundant elements in all samples. The enrichment factors show that elements As, Cd, Cr, Cu, Pb and Zn were significantly enriched in particles, especially in fine particles, posing an adverse impact on human health. This study can be used to assist the development of particle monitoring programmes in the vicinity of industrial areas and also help to establish an elemental modality dataset on the exposure and risk assessments of atmospheric particles.

LanguageEnglish
Article number133534
Number of pages11
JournalScience of the Total Environment
Volume694
DOIs
Publication statusPublished - 1 Dec 2019

Fingerprint

atmospheric particle
Steelmaking
Iron
Air quality
iron
industry
Industry
Particulate Matter
Inductively coupled plasma
Risk assessment
Surface morphology
Aerodynamics
air quality
Particle size
Health
Scanning electron microscopy
Monitoring
X-ray spectroscopy
aerodynamics
particle

Keywords

  • Atmospheric particles
  • Iron and steelmaking
  • Mass analysis
  • Size distribution
  • Elemental analysis

Cite this

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title = "Characterization of size resolved atmospheric particles in the vicinity of iron and steelmaking industries in China",
abstract = "(Graphical abstract)China currently faces environmental challenges of lower air quality, partly as a result of industrial activities. The aim of this study was to investigate the role of iron and steelmaking facilities to regional air quality in four selected industry dominated urban centres in China. Nine different particle size ranges present in atmospheric particles collected from four sites in Kunming (KM), Wuhan (WH), Nanjing (NJ) and Ningbo (NB) were analysed and compared with particles collected at one background site at the Ningbo Nottingham University (UN) with very little industrial influence in China. Similar mass concentration levels of particulate matter PM2.1 and PM1.1 were found at the three sites near older iron and steelmaking plants (KM, WH and NJ). Significantly lower levels of PM2.1 and PM1.1 were collected at the fourth site (NB), which is near to a modern and coastal iron and steelmaking plant. The particles collected had the highest mass concentration in the aerodynamic diameter range of 3.3–9.0 μm for all sites, except for the background site (UN). Scanning electron microscopy equipped with energy-dispersive X-ray spectroscopy, and inductively coupled plasma were used to determine the surface morphology and particle chemistry. Al, Ca, Fe, K, Mg, Na and Zn were found as the most abundant elements in all samples. The enrichment factors show that elements As, Cd, Cr, Cu, Pb and Zn were significantly enriched in particles, especially in fine particles, posing an adverse impact on human health. This study can be used to assist the development of particle monitoring programmes in the vicinity of industrial areas and also help to establish an elemental modality dataset on the exposure and risk assessments of atmospheric particles.",
keywords = "Atmospheric particles, Iron and steelmaking, Mass analysis, Size distribution, Elemental analysis",
author = "Xiaoxia Yang and Xiaoteng Zhou and Tao Kan and Vladimir Strezov and Peter Nelson and Tim Evans and Yijiao Jiang",
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AU - Yang, Xiaoxia

AU - Zhou, Xiaoteng

AU - Kan, Tao

AU - Strezov, Vladimir

AU - Nelson, Peter

AU - Evans, Tim

AU - Jiang, Yijiao

PY - 2019/12/1

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N2 - (Graphical abstract)China currently faces environmental challenges of lower air quality, partly as a result of industrial activities. The aim of this study was to investigate the role of iron and steelmaking facilities to regional air quality in four selected industry dominated urban centres in China. Nine different particle size ranges present in atmospheric particles collected from four sites in Kunming (KM), Wuhan (WH), Nanjing (NJ) and Ningbo (NB) were analysed and compared with particles collected at one background site at the Ningbo Nottingham University (UN) with very little industrial influence in China. Similar mass concentration levels of particulate matter PM2.1 and PM1.1 were found at the three sites near older iron and steelmaking plants (KM, WH and NJ). Significantly lower levels of PM2.1 and PM1.1 were collected at the fourth site (NB), which is near to a modern and coastal iron and steelmaking plant. The particles collected had the highest mass concentration in the aerodynamic diameter range of 3.3–9.0 μm for all sites, except for the background site (UN). Scanning electron microscopy equipped with energy-dispersive X-ray spectroscopy, and inductively coupled plasma were used to determine the surface morphology and particle chemistry. Al, Ca, Fe, K, Mg, Na and Zn were found as the most abundant elements in all samples. The enrichment factors show that elements As, Cd, Cr, Cu, Pb and Zn were significantly enriched in particles, especially in fine particles, posing an adverse impact on human health. This study can be used to assist the development of particle monitoring programmes in the vicinity of industrial areas and also help to establish an elemental modality dataset on the exposure and risk assessments of atmospheric particles.

AB - (Graphical abstract)China currently faces environmental challenges of lower air quality, partly as a result of industrial activities. The aim of this study was to investigate the role of iron and steelmaking facilities to regional air quality in four selected industry dominated urban centres in China. Nine different particle size ranges present in atmospheric particles collected from four sites in Kunming (KM), Wuhan (WH), Nanjing (NJ) and Ningbo (NB) were analysed and compared with particles collected at one background site at the Ningbo Nottingham University (UN) with very little industrial influence in China. Similar mass concentration levels of particulate matter PM2.1 and PM1.1 were found at the three sites near older iron and steelmaking plants (KM, WH and NJ). Significantly lower levels of PM2.1 and PM1.1 were collected at the fourth site (NB), which is near to a modern and coastal iron and steelmaking plant. The particles collected had the highest mass concentration in the aerodynamic diameter range of 3.3–9.0 μm for all sites, except for the background site (UN). Scanning electron microscopy equipped with energy-dispersive X-ray spectroscopy, and inductively coupled plasma were used to determine the surface morphology and particle chemistry. Al, Ca, Fe, K, Mg, Na and Zn were found as the most abundant elements in all samples. The enrichment factors show that elements As, Cd, Cr, Cu, Pb and Zn were significantly enriched in particles, especially in fine particles, posing an adverse impact on human health. This study can be used to assist the development of particle monitoring programmes in the vicinity of industrial areas and also help to establish an elemental modality dataset on the exposure and risk assessments of atmospheric particles.

KW - Atmospheric particles

KW - Iron and steelmaking

KW - Mass analysis

KW - Size distribution

KW - Elemental analysis

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