Effect of dispersion method on the deterioration, interfacial interactions and re-agglomeration of carbon nanotubes in titanium metal matrix composites

Khurram S. Munir, Yuncang Li, Daniel Liang, Ma Qian, Wei Xu, Cuie Wen*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

69 Citations (Scopus)

Abstract

The influence of various synthesis techniques on the dispersion and evolution of multi-walled carbon nanotubes (MWCNTs) in titanium (Ti) metal matrix composites (TMCs) prepared via powder metallurgy routes has been investigated. The synthesis techniques included sonication, high energy ball milling (HEBM), cold compaction, high temperature vacuum sintering and spark plasma sintering (SPS). Powder mixtures of Ti and MWCNTs (0.5wt.%) were processed by HEBM in two batches: (i) ball milling of the mixtures (Batch 1) and (ii) ball milling of Ti powder alone, followed by a further ball milling with sonicated MWCNTs (Batch 2). Both batches of the powder mixtures were pressed at 40MPa into green compacts and then sintered in vacuum. Batch 2 powder mixtures were also consolidated using SPS. The crystallinity and sp2 carbon network of the MWCNTs were characterized through analyzing the characteristic Raman peak ratio (ID/IG) of each processed sample. X-ray diffraction (XRD) was used for phase identification. Scanning electron microscopy (SEM) and transmission electron microscopy (TEM) were used to study the morphology of the MWCNTs in the powder mixtures. The evolution of MWCNTs during the fabrication process and mechanical properties of the sintered compacts were discussed in conjunction with the formation of nano-crystalline TiC.

Original languageEnglish
Pages (from-to)138-148
Number of pages11
JournalMaterials and Design
Volume88
DOIs
Publication statusPublished - 25 Dec 2015
Externally publishedYes

Keywords

  • High energy ball milling (HEBM)
  • Multi-walled carbon nanotubes (MWCNTs)
  • MWCNTs-Ti composites
  • Raman spectroscopy
  • Spark plasma sintering (SPS)

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