First search for pulsed CH maser emission stimulated by a pulsar

We present the first search for pulsed CH maser emission potentially stimulated by PSR J1644-4559, conducted using the ultra-wide-bandwidth low-frequency receiver on Murriyang, CSIRO's Parkes Radio Telescope. Observations targeted three CH Λ-doublet transitions at 3264, 3335, and 3349 MHz, with a variability timescale of 78 ms. We detected ten CH emission features at 3335 and 3349 MHz, and seven features at 3264 MHz, during both pulsar-ON and pulsar-OFF phases. The observed velocities align with the OH emission and absorption reported by a previous study, suggesting a close spatial association between CH and OH molecules. The derived column densities for CH clouds within the Parkes beam range from 0.05 to 9.8 × 10¹³ cm⁻², indicating that these clouds are likely in diffuse and translucent states. Upper limits for CH column densities within the pulsar beam ranged from 0.3 to 9.8 × 10¹³ cm⁻². Comparison of these column densities suggests that CH clouds may exhibit clumpiness and substructure. No significant stimulated emission feature was detected in the optical depth spectra. Additionally, as part of our search for pulsed stimulated emission, we investigated the potential CH absorption of the pulsar signal and found none, in agreement with astrophysical expectations. The upper limits for the potential maser amplification factors towards PSR J1644-4559 at 3264, 3335, and 3349 MHz are 1.014, 1.009, and 1.009, respectively. This study demonstrates the feasibility of detecting pulsed CH maser emission in the interstellar medium stimulated by pulsar photons.