Linear and nonlinear optics of hybrid plexitonic nanosystems

Dzmitry Melnikau, Ruben Esteban, Alexander A. Govyadinov, Diana Savateeva, Thomas Simon, Ana Sánchez-Iglesias, Marek Grzelczak, Mikolaj K. Schmidt, Alexander S. Urban, Luis M. Liz-Marzan, Jochen Feldmann, Javier Aizpurua, Yury P. Rakovich*

*Corresponding author for this work

Research output: Chapter in Book/Report/Conference proceedingConference proceeding contributionpeer-review

Abstract

We report our recent results of investigation of the interactions between localized plasmons in gold nanorods and excitons in J-aggregates. We were able to track an anticrossing behavior of the hybridized modes both in the extinction and in the photoluminescence spectra of this hybrid system. We identified the nonlinear optical behavior of this system by transient absorption spectroscopy. Finally using magnetic circular dichroism spectroscopy, we show that nonmagnetic organic molecules exhibit magneto-optical response due to binding to a plasmonic nanoparticles. In our experiments, we also studied the effect of detuning as well as the effect of off- and on resonance excitation on the hybrid states.

Original languageEnglish
Title of host publication2017 19th International Conference on Transparent Optical Networks (ICTON)
Place of PublicationPiscataway, NJ, USA
PublisherInstitute of Electrical and Electronics Engineers (IEEE)
Pages1-5
Number of pages5
ISBN (Electronic)9781538608593
ISBN (Print)9781538608609
DOIs
Publication statusPublished - 1 Sep 2017
Externally publishedYes
Event19th International Conference on Transparent Optical Networks, ICTON 2017 - Girona, Catalonia, Spain
Duration: 2 Jul 20176 Jul 2017

Conference

Conference19th International Conference on Transparent Optical Networks, ICTON 2017
CountrySpain
CityGirona, Catalonia
Period2/07/176/07/17

Keywords

  • excitons
  • magneto-optical effect
  • nonlinear effects
  • plasmons
  • Rabi splitting
  • strong coupling

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