Linear and nonlinear optics of hybrid plexitonic nanosystems

Dzmitry Melnikau; Ruben Esteban; Alexander A. Govyadinov; Diana Savateeva; Thomas Simon; Ana Sánchez-Iglesias; Marek Grzelczak; Mikolaj K. Schmidt; Alexander S. Urban; Luis M. Liz-Marzan; Jochen Feldmann; Javier Aizpurua; Yury P. Rakovich

doi:10.1109/ICTON.2017.8025078

Linear and nonlinear optics of hybrid plexitonic nanosystems

Dzmitry Melnikau, Ruben Esteban, Alexander A. Govyadinov, Diana Savateeva, Thomas Simon, Ana Sánchez-Iglesias, Marek Grzelczak, Mikolaj K. Schmidt, Alexander S. Urban, Luis M. Liz-Marzan, Jochen Feldmann, Javier Aizpurua, Yury P. Rakovich^*

^*Corresponding author for this work

Research output: Chapter in Book/Report/Conference proceeding › Conference proceeding contribution › peer-review

Abstract

We report our recent results of investigation of the interactions between localized plasmons in gold nanorods and excitons in J-aggregates. We were able to track an anticrossing behavior of the hybridized modes both in the extinction and in the photoluminescence spectra of this hybrid system. We identified the nonlinear optical behavior of this system by transient absorption spectroscopy. Finally using magnetic circular dichroism spectroscopy, we show that nonmagnetic organic molecules exhibit magneto-optical response due to binding to a plasmonic nanoparticles. In our experiments, we also studied the effect of detuning as well as the effect of off- and on resonance excitation on the hybrid states.

Original language	English
Title of host publication	2017 19th International Conference on Transparent Optical Networks (ICTON)
Place of Publication	Piscataway, NJ, USA
Publisher	Institute of Electrical and Electronics Engineers (IEEE)
Pages	1-5
Number of pages	5
ISBN (Electronic)	9781538608593
ISBN (Print)	9781538608609
DOIs	https://doi.org/10.1109/ICTON.2017.8025078
Publication status	Published - 1 Sept 2017
Externally published	Yes
Event	19th International Conference on Transparent Optical Networks, ICTON 2017 - Girona, Catalonia, Spain Duration: 2 Jul 2017 → 6 Jul 2017

Conference

Conference	19th International Conference on Transparent Optical Networks, ICTON 2017
Country/Territory	Spain
City	Girona, Catalonia
Period	2/07/17 → 6/07/17

Keywords

excitons
magneto-optical effect
nonlinear effects
plasmons
Rabi splitting
strong coupling

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10.1109/ICTON.2017.8025078

Cite this

Melnikau, D., Esteban, R., Govyadinov, A. A., Savateeva, D., Simon, T., Sánchez-Iglesias, A., Grzelczak, M., Schmidt, M. K., Urban, A. S., Liz-Marzan, L. M., Feldmann, J., Aizpurua, J., & Rakovich, Y. P. (2017). Linear and nonlinear optics of hybrid plexitonic nanosystems. In 2017 19th International Conference on Transparent Optical Networks (ICTON) (pp. 1-5). Article 8025078 Institute of Electrical and Electronics Engineers (IEEE). https://doi.org/10.1109/ICTON.2017.8025078

@inproceedings{c51c03d68d5a4f94bb708028f65c5879,

title = "Linear and nonlinear optics of hybrid plexitonic nanosystems",

abstract = "We report our recent results of investigation of the interactions between localized plasmons in gold nanorods and excitons in J-aggregates. We were able to track an anticrossing behavior of the hybridized modes both in the extinction and in the photoluminescence spectra of this hybrid system. We identified the nonlinear optical behavior of this system by transient absorption spectroscopy. Finally using magnetic circular dichroism spectroscopy, we show that nonmagnetic organic molecules exhibit magneto-optical response due to binding to a plasmonic nanoparticles. In our experiments, we also studied the effect of detuning as well as the effect of off- and on resonance excitation on the hybrid states.",

keywords = "excitons, magneto-optical effect, nonlinear effects, plasmons, Rabi splitting, strong coupling",

author = "Dzmitry Melnikau and Ruben Esteban and Govyadinov, \{Alexander A.\} and Diana Savateeva and Thomas Simon and Ana S{\'a}nchez-Iglesias and Marek Grzelczak and Schmidt, \{Mikolaj K.\} and Urban, \{Alexander S.\} and Liz-Marzan, \{Luis M.\} and Jochen Feldmann and Javier Aizpurua and Rakovich, \{Yury P.\}",

year = "2017",

month = sep,

day = "1",

doi = "10.1109/ICTON.2017.8025078",

language = "English",

isbn = "9781538608609",

pages = "1--5",

booktitle = "2017 19th International Conference on Transparent Optical Networks (ICTON)",

publisher = "Institute of Electrical and Electronics Engineers (IEEE)",

address = "United States",

note = "19th International Conference on Transparent Optical Networks, ICTON 2017 ; Conference date: 02-07-2017 Through 06-07-2017",

}

Melnikau, D, Esteban, R, Govyadinov, AA, Savateeva, D, Simon, T, Sánchez-Iglesias, A, Grzelczak, M, Schmidt, MK, Urban, AS, Liz-Marzan, LM, Feldmann, J, Aizpurua, J & Rakovich, YP 2017, Linear and nonlinear optics of hybrid plexitonic nanosystems. in 2017 19th International Conference on Transparent Optical Networks (ICTON) ., 8025078, Institute of Electrical and Electronics Engineers (IEEE), Piscataway, NJ, USA, pp. 1-5, 19th International Conference on Transparent Optical Networks, ICTON 2017, Girona, Catalonia, Spain, 2/07/17. https://doi.org/10.1109/ICTON.2017.8025078

Linear and nonlinear optics of hybrid plexitonic nanosystems. / Melnikau, Dzmitry; Esteban, Ruben; Govyadinov, Alexander A. et al.
2017 19th International Conference on Transparent Optical Networks (ICTON) . Piscataway, NJ, USA: Institute of Electrical and Electronics Engineers (IEEE), 2017. p. 1-5 8025078.

Research output: Chapter in Book/Report/Conference proceeding › Conference proceeding contribution › peer-review

TY - GEN

T1 - Linear and nonlinear optics of hybrid plexitonic nanosystems

AU - Melnikau, Dzmitry

AU - Esteban, Ruben

AU - Govyadinov, Alexander A.

AU - Savateeva, Diana

AU - Simon, Thomas

AU - Sánchez-Iglesias, Ana

AU - Grzelczak, Marek

AU - Schmidt, Mikolaj K.

AU - Urban, Alexander S.

AU - Liz-Marzan, Luis M.

AU - Feldmann, Jochen

AU - Aizpurua, Javier

AU - Rakovich, Yury P.

PY - 2017/9/1

Y1 - 2017/9/1

N2 - We report our recent results of investigation of the interactions between localized plasmons in gold nanorods and excitons in J-aggregates. We were able to track an anticrossing behavior of the hybridized modes both in the extinction and in the photoluminescence spectra of this hybrid system. We identified the nonlinear optical behavior of this system by transient absorption spectroscopy. Finally using magnetic circular dichroism spectroscopy, we show that nonmagnetic organic molecules exhibit magneto-optical response due to binding to a plasmonic nanoparticles. In our experiments, we also studied the effect of detuning as well as the effect of off- and on resonance excitation on the hybrid states.

AB - We report our recent results of investigation of the interactions between localized plasmons in gold nanorods and excitons in J-aggregates. We were able to track an anticrossing behavior of the hybridized modes both in the extinction and in the photoluminescence spectra of this hybrid system. We identified the nonlinear optical behavior of this system by transient absorption spectroscopy. Finally using magnetic circular dichroism spectroscopy, we show that nonmagnetic organic molecules exhibit magneto-optical response due to binding to a plasmonic nanoparticles. In our experiments, we also studied the effect of detuning as well as the effect of off- and on resonance excitation on the hybrid states.

KW - excitons

KW - magneto-optical effect

KW - nonlinear effects

KW - plasmons

KW - Rabi splitting

KW - strong coupling

UR - https://www.scopus.com/pages/publications/85031031627

U2 - 10.1109/ICTON.2017.8025078

DO - 10.1109/ICTON.2017.8025078

M3 - Conference proceeding contribution

AN - SCOPUS:85031031627

SN - 9781538608609

SP - 1

EP - 5

BT - 2017 19th International Conference on Transparent Optical Networks (ICTON)

PB - Institute of Electrical and Electronics Engineers (IEEE)

CY - Piscataway, NJ, USA

T2 - 19th International Conference on Transparent Optical Networks, ICTON 2017

Y2 - 2 July 2017 through 6 July 2017

ER -

Linear and nonlinear optics of hybrid plexitonic nanosystems

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Keywords

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