Abstract
We report on the observation of nonlinear optical excitation and related photoluminescence from single InP semiconductor nanowires held in suspension using a gradient force optical tweezers. Photoexcitation of free carriers is achieved through absorption of infrared (1.17 eV) photons from the trapping source via a combination of two- and three-photon processes. This was confirmed by power-dependent photoluminescence measurements. Marked differences in spectral features are noted between nonlinear optical excitation and direct excitation and are related to band-filling effects. Direct observation of second harmonic generation in trapped InP nanowires confirms the presence of nonlinear optical processes.
| Original language | English |
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| Pages (from-to) | 4149-4153 |
| Number of pages | 5 |
| Journal | Nano Letters |
| Volume | 11 |
| Issue number | 10 |
| DOIs | |
| Publication status | Published - 12 Oct 2011 |