Abstract
Nonlinear conversion of unpolarized beams to lower frequencies is generally inefficient in χ(2) materials, as it is challenging to achieve phase-matching for input ordinary and extraordinary beams simultaneously in the normal dispersion regime. Here, we show that cubic Raman crystals having doubly and triply degenerate (E and F type) modes provide a method for efficient nonlinear frequency downconversion of an unpolarized beam and yield a linearly polarized output state. Using Mueller calculus, optimal crystal directions for such polarization conversion are determined. Using diamond, an example of an F-class Raman crystal, we have verified that such conversion is possible with near quantum-defect-limited slope efficiency and a linear polarization contrast of more than 23.9 dB.
Original language | English |
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Article number | 41702 |
Pages (from-to) | 1-8 |
Number of pages | 8 |
Journal | Scientific Reports |
Volume | 7 |
DOIs | |
Publication status | Published - 7 Feb 2017 |