TY - JOUR
T1 - Recent increase in Antarctic Peninsula ice core uranium concentrations
AU - Potocki, Mariusz
AU - Mayewski, Paul A.
AU - Kurbatov, Andrei V.
AU - Simões, Jefferson C.
AU - Dixon, Daniel A.
AU - Goodwin, Ian
AU - Carleton, Andrew M.
AU - Handley, Michael J.
AU - Jaña, Ricardo
AU - Korotkikh, Elena V.
N1 - Copyright the Author(s) 2016. Version archived for private and non-commercial use with the permission of the author/s and according to publisher conditions. For further rights please contact the publisher.
PY - 2016/9/1
Y1 - 2016/9/1
N2 - Understanding the distribution of airborne uranium is important because it can result in both chemical and radiological toxicity. Ice cores offer the most robust reconstruction of past atmospheric levels of toxic substances. Here we present the first sub-annually dated, continuously sampled ice core documenting change in U levels in the Southern Hemisphere. The ice core was recovered from the Detroit Plateau, northern Antarctic Peninsula, in 2007 by a joint Brazilian-Chilean-US team. It displays a significant increase in U concentration that coincides with reported mining activities in the Southern Hemisphere, notably Australia. Raw U concentrations in the Detroit Plateau ice core increased by as much as 102 between the 1980s and 2000s accompanied by increased variability in recent years. Decadal mean U concentrations increased by a factor of ~3 from 1980 to 2007, reaching a mean of 205 pg/L from 2000 to 2007. The fact that other terrestrial source dust elements such as Ce, La, Pr, and Ti do not show a similar increase and that the increased U concentrations are enriched above natural crustal levels, supports an anthropogenic source for the U as opposed to a change in atmospheric circulation.
AB - Understanding the distribution of airborne uranium is important because it can result in both chemical and radiological toxicity. Ice cores offer the most robust reconstruction of past atmospheric levels of toxic substances. Here we present the first sub-annually dated, continuously sampled ice core documenting change in U levels in the Southern Hemisphere. The ice core was recovered from the Detroit Plateau, northern Antarctic Peninsula, in 2007 by a joint Brazilian-Chilean-US team. It displays a significant increase in U concentration that coincides with reported mining activities in the Southern Hemisphere, notably Australia. Raw U concentrations in the Detroit Plateau ice core increased by as much as 102 between the 1980s and 2000s accompanied by increased variability in recent years. Decadal mean U concentrations increased by a factor of ~3 from 1980 to 2007, reaching a mean of 205 pg/L from 2000 to 2007. The fact that other terrestrial source dust elements such as Ce, La, Pr, and Ti do not show a similar increase and that the increased U concentrations are enriched above natural crustal levels, supports an anthropogenic source for the U as opposed to a change in atmospheric circulation.
UR - http://www.scopus.com/inward/record.url?scp=84974623798&partnerID=8YFLogxK
U2 - 10.1016/j.atmosenv.2016.06.010
DO - 10.1016/j.atmosenv.2016.06.010
M3 - Article
AN - SCOPUS:84974623798
SN - 1352-2310
VL - 140
SP - 381
EP - 385
JO - Atmospheric Environment
JF - Atmospheric Environment
ER -