Rotationally resolved Raman-optical double resonance with fluorescence detection

D. A. King; R. Haines; N. R. Isenor; B. J. Orr

doi:10.1364/OL.8.000629

Rotationally resolved Raman-optical double resonance with fluorescence detection

D. A. King, R. Haines, N. R. Isenor^*, B. J. Orr

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

20 Citations (Scopus)

Abstract

A pulsed excitation sequence, consisting of coherent Raman pumping of a molecular rovibrational transition followed by rovibronic probing through visible laser-induced fluorescence, is used in Raman-optical double resonance studies of D₂CO. The experiments demonstrate enhanced sensitivity, with respect to conventional coherent Raman spectroscopy, and enable individual 0- and P-branch Raman transitions to be distinguished with high specificity under effectively collision-free conditions.

Original language	English
Pages (from-to)	629-631
Number of pages	3
Journal	Optics Letters
Volume	8
Issue number	12
DOIs	https://doi.org/10.1364/OL.8.000629
Publication status	Published - 1983
Externally published	Yes

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title = "Rotationally resolved Raman-optical double resonance with fluorescence detection",

abstract = "A pulsed excitation sequence, consisting of coherent Raman pumping of a molecular rovibrational transition followed by rovibronic probing through visible laser-induced fluorescence, is used in Raman-optical double resonance studies of D2CO. The experiments demonstrate enhanced sensitivity, with respect to conventional coherent Raman spectroscopy, and enable individual 0- and P-branch Raman transitions to be distinguished with high specificity under effectively collision-free conditions.",

author = "King, {D. A.} and R. Haines and Isenor, {N. R.} and Orr, {B. J.}",

year = "1983",

doi = "10.1364/OL.8.000629",

language = "English",

volume = "8",

pages = "629--631",

journal = "Optics Letters",

issn = "0146-9592",

publisher = "OPTICAL SOC AMER",

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T1 - Rotationally resolved Raman-optical double resonance with fluorescence detection

AU - King, D. A.

AU - Haines, R.

AU - Isenor, N. R.

AU - Orr, B. J.

PY - 1983

Y1 - 1983

N2 - A pulsed excitation sequence, consisting of coherent Raman pumping of a molecular rovibrational transition followed by rovibronic probing through visible laser-induced fluorescence, is used in Raman-optical double resonance studies of D2CO. The experiments demonstrate enhanced sensitivity, with respect to conventional coherent Raman spectroscopy, and enable individual 0- and P-branch Raman transitions to be distinguished with high specificity under effectively collision-free conditions.

AB - A pulsed excitation sequence, consisting of coherent Raman pumping of a molecular rovibrational transition followed by rovibronic probing through visible laser-induced fluorescence, is used in Raman-optical double resonance studies of D2CO. The experiments demonstrate enhanced sensitivity, with respect to conventional coherent Raman spectroscopy, and enable individual 0- and P-branch Raman transitions to be distinguished with high specificity under effectively collision-free conditions.

UR - http://www.scopus.com/inward/record.url?scp=84975598524&partnerID=8YFLogxK

U2 - 10.1364/OL.8.000629

DO - 10.1364/OL.8.000629

M3 - Article

AN - SCOPUS:84975598524

SN - 0146-9592

VL - 8

SP - 629

EP - 631

JO - Optics Letters

JF - Optics Letters

IS - 12

ER -

Rotationally resolved Raman-optical double resonance with fluorescence detection

Abstract

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