Rotationally resolved Raman-optical double resonance with fluorescence detection

D. A. King, R. Haines, N. R. Isenor*, B. J. Orr

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

20 Citations (Scopus)


A pulsed excitation sequence, consisting of coherent Raman pumping of a molecular rovibrational transition followed by rovibronic probing through visible laser-induced fluorescence, is used in Raman-optical double resonance studies of D2CO. The experiments demonstrate enhanced sensitivity, with respect to conventional coherent Raman spectroscopy, and enable individual 0- and P-branch Raman transitions to be distinguished with high specificity under effectively collision-free conditions.

Original languageEnglish
Pages (from-to)629-631
Number of pages3
JournalOptics Letters
Issue number12
Publication statusPublished - 1983
Externally publishedYes


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