Abstract
A pulsed excitation sequence, consisting of coherent Raman pumping of a molecular rovibrational transition followed by rovibronic probing through visible laser-induced fluorescence, is used in Raman-optical double resonance studies of D2CO. The experiments demonstrate enhanced sensitivity, with respect to conventional coherent Raman spectroscopy, and enable individual 0- and P-branch Raman transitions to be distinguished with high specificity under effectively collision-free conditions.
| Original language | English |
|---|---|
| Pages (from-to) | 629-631 |
| Number of pages | 3 |
| Journal | Optics Letters |
| Volume | 8 |
| Issue number | 12 |
| DOIs | |
| Publication status | Published - 1983 |
| Externally published | Yes |
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