Sequential deposition of CH3NH3PbI3 on planar NiO film for efficient planar perovskite solar cells

Long Hu; Jun Peng; Weiwei Wang; Zhe Xia; Jianyu Yuan; Jialing Lu; Xiaodong Huang; Wanli Ma; Huaibing Song; Wei Chen; Yi-Bing Cheng; Jiang Tang

doi:10.1021/ph5000067

Sequential deposition of CH₃NH₃PbI₃ on planar NiO film for efficient planar perovskite solar cells

Long Hu, Jun Peng, Weiwei Wang, Zhe Xia, Jianyu Yuan, Jialing Lu, Xiaodong Huang, Wanli Ma^*, Huaibing Song, Wei Chen, Yi-Bing Cheng, Jiang Tang^*

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

262 Citations (Scopus)

Abstract

The new emerging organometal trihalide perovskite holds great potential for high-efficiency, low-cost solar cells because of its high solar to electricity conversation efficiency (>16%) achieved within 4 years of research and its low-temperature solution processing. In this Letter we introduce NiO as the hole-collecting and -conducting layer in perovskite solar cells. Through a modified sequential deposition strategy, we successfully fabricated high-quality CH₃NH₃PbI₃ onto a planar NiO layer and built a planar inverted ITO/NiO/CH₃NH₃PbI₃/PCBM/Al photovoltaic device. A device efficiency of 7.6% was achieved with an impressively high open-circuit voltage (V_oc) of 1.05 V. Our study demonstrates the potential application of a deep work function NiO layer for perovskite solar cells.

[Graph presented]

Original language	English
Pages (from-to)	547-553
Number of pages	7
Journal	ACS Photonics
Volume	1
Issue number	7
DOIs	https://doi.org/10.1021/ph5000067
Publication status	Published - 16 Jul 2014
Externally published	Yes

Keywords

perovskite
solar cell
NiO
sequential deposition

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10.1021/ph5000067

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@article{22fdb83204df43af9e4a256b1b4b8eb7,

title = "Sequential deposition of CH3NH3PbI3 on planar NiO film for efficient planar perovskite solar cells",

abstract = "The new emerging organometal trihalide perovskite holds great potential for high-efficiency, low-cost solar cells because of its high solar to electricity conversation efficiency (>16\%) achieved within 4 years of research and its low-temperature solution processing. In this Letter we introduce NiO as the hole-collecting and -conducting layer in perovskite solar cells. Through a modified sequential deposition strategy, we successfully fabricated high-quality CH3NH3PbI3 onto a planar NiO layer and built a planar inverted ITO/NiO/CH3NH3PbI3/PCBM/Al photovoltaic device. A device efficiency of 7.6\% was achieved with an impressively high open-circuit voltage (Voc) of 1.05 V. Our study demonstrates the potential application of a deep work function NiO layer for perovskite solar cells. [Graph presented]",

keywords = "perovskite, solar cell, NiO, sequential deposition",

author = "Long Hu and Jun Peng and Weiwei Wang and Zhe Xia and Jianyu Yuan and Jialing Lu and Xiaodong Huang and Wanli Ma and Huaibing Song and Wei Chen and Yi-Bing Cheng and Jiang Tang",

year = "2014",

month = jul,

day = "16",

doi = "10.1021/ph5000067",

language = "English",

volume = "1",

pages = "547--553",

journal = "ACS Photonics",

issn = "2330-4022",

publisher = "American Chemical Society",

number = "7",

}

TY - JOUR

T1 - Sequential deposition of CH3NH3PbI3 on planar NiO film for efficient planar perovskite solar cells

AU - Hu, Long

AU - Peng, Jun

AU - Wang, Weiwei

AU - Xia, Zhe

AU - Yuan, Jianyu

AU - Lu, Jialing

AU - Huang, Xiaodong

AU - Ma, Wanli

AU - Song, Huaibing

AU - Chen, Wei

AU - Cheng, Yi-Bing

AU - Tang, Jiang

PY - 2014/7/16

Y1 - 2014/7/16

N2 - The new emerging organometal trihalide perovskite holds great potential for high-efficiency, low-cost solar cells because of its high solar to electricity conversation efficiency (>16%) achieved within 4 years of research and its low-temperature solution processing. In this Letter we introduce NiO as the hole-collecting and -conducting layer in perovskite solar cells. Through a modified sequential deposition strategy, we successfully fabricated high-quality CH3NH3PbI3 onto a planar NiO layer and built a planar inverted ITO/NiO/CH3NH3PbI3/PCBM/Al photovoltaic device. A device efficiency of 7.6% was achieved with an impressively high open-circuit voltage (Voc) of 1.05 V. Our study demonstrates the potential application of a deep work function NiO layer for perovskite solar cells. [Graph presented]

AB - The new emerging organometal trihalide perovskite holds great potential for high-efficiency, low-cost solar cells because of its high solar to electricity conversation efficiency (>16%) achieved within 4 years of research and its low-temperature solution processing. In this Letter we introduce NiO as the hole-collecting and -conducting layer in perovskite solar cells. Through a modified sequential deposition strategy, we successfully fabricated high-quality CH3NH3PbI3 onto a planar NiO layer and built a planar inverted ITO/NiO/CH3NH3PbI3/PCBM/Al photovoltaic device. A device efficiency of 7.6% was achieved with an impressively high open-circuit voltage (Voc) of 1.05 V. Our study demonstrates the potential application of a deep work function NiO layer for perovskite solar cells. [Graph presented]

KW - perovskite

KW - solar cell

KW - NiO

KW - sequential deposition

UR - https://www.scopus.com/pages/publications/84908021027

U2 - 10.1021/ph5000067

DO - 10.1021/ph5000067

M3 - Article

AN - SCOPUS:84908021027

SN - 2330-4022

VL - 1

SP - 547

EP - 553

JO - ACS Photonics

JF - ACS Photonics

IS - 7

ER -

Sequential deposition of CH₃NH₃PbI₃ on planar NiO film for efficient planar perovskite solar cells

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Keywords

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