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Synergistic barium titanate/MXene composite as a high-performance piezo-photocatalyst for efficient dye degradation

Linghui Meng, Lu Zhou, Chao Liu, Haowei Jia, Yile Lu, Dali Ji, Tianyue Liang, Yu Yuan, Xinren Zhang, Yanzhe Zhu, Yue Jiang, Peiyuan Guan*, Yingze Zhou*, Qi Zhang, Tao Wan, Mengyao Li*, Zhi Li, Rakesh Joshi, Zhaojun Han, Dewei Chu*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

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Abstract

[Graphical abstract presents]

Piezo-photocatalysis combines photocatalysis and piezoelectric effects to enhance catalytic efficiency by creating an internal electric field in the photocatalyst, improving carrier separation and overall performance. This study presents a high-performance piezo-photocatalyst for efficient dye degradation using a synergistic barium titanate (BTO)-MXene composite. The composite was synthesized via a facile method, combining the unique properties of BTO nanoparticles with the high conductivity of MXene. The structural and morphological analysis confirmed the successful formation of the composite, with well-dispersed BTO nanoparticles on the MXene surface. The piezo-photocatalytic activity of the composite was evaluated using a typical dye solution (Rhodamine B: RhB) under ultraviolet irradiation and mechanical agitation. The results revealed a remarkable enhancement in dye degradation (90 % in 15 min for piezo-photocatalysis) compared to individual stimuli (58.2 % for photocatalysis and 95.8 % in 90 min for piezocatalysis), highlighting the synergistic effects between BTO and MXene. The enhanced catalytic performance was attributed to the efficient charge separation and transfer facilitated by the composite's structure, leading to increased reactive species generation and dye molecule degradation. Furthermore, the composite exhibited excellent stability and reusability, showcasing its potential for practical applications in wastewater treatment. Overall, this work represents a promising strategy for designing high-performance synergistic catalysts, addressing the pressing need for sustainable solutions in environmental remediation.

Original languageEnglish
Pages (from-to)972-981
Number of pages10
JournalJournal of Colloid and Interface Science
Volume674
DOIs
Publication statusPublished - 15 Nov 2024
Externally publishedYes

Bibliographical note

Copyright the Author(s) 2024. Version archived for private and non-commercial use with the permission of the author/s and according to publisher conditions. For further rights please contact the publisher.

Keywords

  • Synergistic catalysis
  • Piezocatalysis
  • Photocatalysis
  • Dye degradation
  • Advanced oxidizing process

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