Time-resolved vacuum-ultraviolet emission (λ = 60-120 nm) from a high pressure DBD-excited helium plasma: formation mechanisms of the fast component

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Abstract

We report time and wavelength resolved studies of the vacuum-ultraviolet (VUV) emission from a windowless dielectric barrier discharge (DBD) in helium. Short-pulse voltage excitation is utilised to clearly resolve the fast and slow temporal components of the Hopfield continuum between λ = 60-120 nm. Experimental results and theoretical modelling of the spectral distributions indicate that the two components of the VUV emission must originate from the same radiating molecular state - , and that two distinct pumping mechanisms populate this state. The time evolution of the fast component is found to correlate with that from the (0,0) molecular transition (λ = 513.4 nm). Thus the state is initially rapidly pumped via radiative cascade from higher molecular states. In addition, the observed band emissions from the molecular v=0 and v=0 states and the line emissions from the atomic He(n = 3) states all exhibit similar temporal behaviour during the discharge excitation period. Our results are consistent with the recent report of Frost et al (J. Phys. B 34 1569 2001) concerning the existence of a so-called 'neglected channel' to fast production from He(n = 3) atomic state precursors.

LanguageEnglish
Article number085201
Pages1-18
Number of pages18
JournalJournal of Physics D: Applied Physics
Volume49
Issue number8
DOIs
Publication statusPublished - 2 Mar 2016

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helium plasma
Helium
ultraviolet emission
Vacuum
Plasmas
vacuum
Wavelength
excitation
cascades
pumping
Electric potential
helium
continuums
electric potential
pulses
wavelengths

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title = "Time-resolved vacuum-ultraviolet emission (λ = 60-120 nm) from a high pressure DBD-excited helium plasma: formation mechanisms of the fast component",
abstract = "We report time and wavelength resolved studies of the vacuum-ultraviolet (VUV) emission from a windowless dielectric barrier discharge (DBD) in helium. Short-pulse voltage excitation is utilised to clearly resolve the fast and slow temporal components of the Hopfield continuum between λ = 60-120 nm. Experimental results and theoretical modelling of the spectral distributions indicate that the two components of the VUV emission must originate from the same radiating molecular state - , and that two distinct pumping mechanisms populate this state. The time evolution of the fast component is found to correlate with that from the (0,0) molecular transition (λ = 513.4 nm). Thus the state is initially rapidly pumped via radiative cascade from higher molecular states. In addition, the observed band emissions from the molecular v=0 and v=0 states and the line emissions from the atomic He∗(n = 3) states all exhibit similar temporal behaviour during the discharge excitation period. Our results are consistent with the recent report of Frost et al (J. Phys. B 34 1569 2001) concerning the existence of a so-called 'neglected channel' to fast production from He∗(n = 3) atomic state precursors.",
author = "Carman, {R. J.} and R. Ganesan and Kane, {D. M.}",
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language = "English",
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Time-resolved vacuum-ultraviolet emission (λ = 60-120 nm) from a high pressure DBD-excited helium plasma : formation mechanisms of the fast component. / Carman, R. J.; Ganesan, R.; Kane, D. M.

In: Journal of Physics D: Applied Physics, Vol. 49, No. 8, 085201, 02.03.2016, p. 1-18.

Research output: Contribution to journalArticleResearchpeer-review

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T2 - Journal of Physics D: Applied Physics

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AU - Kane, D. M.

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N2 - We report time and wavelength resolved studies of the vacuum-ultraviolet (VUV) emission from a windowless dielectric barrier discharge (DBD) in helium. Short-pulse voltage excitation is utilised to clearly resolve the fast and slow temporal components of the Hopfield continuum between λ = 60-120 nm. Experimental results and theoretical modelling of the spectral distributions indicate that the two components of the VUV emission must originate from the same radiating molecular state - , and that two distinct pumping mechanisms populate this state. The time evolution of the fast component is found to correlate with that from the (0,0) molecular transition (λ = 513.4 nm). Thus the state is initially rapidly pumped via radiative cascade from higher molecular states. In addition, the observed band emissions from the molecular v=0 and v=0 states and the line emissions from the atomic He∗(n = 3) states all exhibit similar temporal behaviour during the discharge excitation period. Our results are consistent with the recent report of Frost et al (J. Phys. B 34 1569 2001) concerning the existence of a so-called 'neglected channel' to fast production from He∗(n = 3) atomic state precursors.

AB - We report time and wavelength resolved studies of the vacuum-ultraviolet (VUV) emission from a windowless dielectric barrier discharge (DBD) in helium. Short-pulse voltage excitation is utilised to clearly resolve the fast and slow temporal components of the Hopfield continuum between λ = 60-120 nm. Experimental results and theoretical modelling of the spectral distributions indicate that the two components of the VUV emission must originate from the same radiating molecular state - , and that two distinct pumping mechanisms populate this state. The time evolution of the fast component is found to correlate with that from the (0,0) molecular transition (λ = 513.4 nm). Thus the state is initially rapidly pumped via radiative cascade from higher molecular states. In addition, the observed band emissions from the molecular v=0 and v=0 states and the line emissions from the atomic He∗(n = 3) states all exhibit similar temporal behaviour during the discharge excitation period. Our results are consistent with the recent report of Frost et al (J. Phys. B 34 1569 2001) concerning the existence of a so-called 'neglected channel' to fast production from He∗(n = 3) atomic state precursors.

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